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A review of covalent organic framework electrode materials for rechargeable metal-ion batteries

ZENG Shu-mao HUANG Xiao-xiong MA Ying-jie ZHI Lin-jie

曾术茂, 黄小雄, 马英杰, 智林杰. 用于可充电金属离子电池的共价有机框架电极材料综述. 新型炭材料, 2021, 36(1): 1-18. doi: 10.1016/S1872-5805(21)60001-X
引用本文: 曾术茂, 黄小雄, 马英杰, 智林杰. 用于可充电金属离子电池的共价有机框架电极材料综述. 新型炭材料, 2021, 36(1): 1-18. doi: 10.1016/S1872-5805(21)60001-X
ZENG Shu-mao, HUANG Xiao-xiong, MA Ying-jie, ZHI Lin-jie. A review of covalent organic framework electrode materials for rechargeable metal-ion batteries. New Carbon Mater., 2021, 36(1): 1-18. doi: 10.1016/S1872-5805(21)60001-X
Citation: ZENG Shu-mao, HUANG Xiao-xiong, MA Ying-jie, ZHI Lin-jie. A review of covalent organic framework electrode materials for rechargeable metal-ion batteries. New Carbon Mater., 2021, 36(1): 1-18. doi: 10.1016/S1872-5805(21)60001-X

用于可充电金属离子电池的共价有机框架电极材料综述

doi: 10.1016/S1872-5805(21)60001-X
详细信息
  • 中图分类号: TQ127.1 + 1

A review of covalent organic framework electrode materials for rechargeable metal-ion batteries

Funds: The Authors would like to offer special thanks to National Natural Science Foundation of China (51425302, 51302045) and the Beijing Natural Science Foundation (2182086)
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    Author Bio:

    †These authors contributed equally to this work

    Corresponding author: MA Ying-jie, Assistant researcher. E-mail: mayj@nanoctr.cnZHI Lin-jie, Professor. E-mail: zhilj@nanoctr.cn
  • †These authors contributed equally to this work. †曾术茂,黄小雄为共同第一作者
  • 摘要: 共价有机框架具有强健的骨架、丰富的电化学活性位点、便于金属离子传输的可控孔道以及利于优化电化学性能的可调控的分子结构,因此是理想的下一代可充电金属离子电池电极材料。此外,共价有机框架电极材料没有传统无机电极材料价格昂贵及含有毒金属的问题,也不存在有机小分子循环稳定性差的问题,在下一代可充电金属离子电池中具有巨大的应用潜力。因此,本文总结了共价有机框架电极材料的电化学活性位点,并着重讨论了通过调节共价有机框架的骨架结构、孔道、活性位点和电子结构提高共价有机框架电极材料电化学性能(包括:能量密度、倍率性能和循环寿命)的策略。为了开发高性能的共价有机框架电极材料,未来的工作需着重于优化它们的离子和电子导电性,进一步提高它们的工作电压以及探明它们的储能机制。本文将有助于开发用于下一代金属离子电池的高性能共价有机框架电极材料。
    †These authors contributed equally to this work. †曾术茂,黄小雄为共同第一作者
  • Figure  1.  Various electrochemical active sites in reported COFs and corresponding theoretical specific capacity (Cth)[52-62]. (a, b, f) reproduced by permission of Nature Publishing Group, (c, d, g, k) reproduced by permission of Wiley-VCH, (e) reproduced by permission of the Royal Society of Chemistry and (h, i, j) reproduced by permission of American Chemical Society.

    Figure  2.  The composite COF@CNT electrode[57]: (a) structure of the COF, (b) interlayer spacing expansion, (c) the cyclic voltammetry curves and (d) the electrochemical performance of the composite electrode (Reproduced by permission of Nature Publishing Group).

    Figure  3.  (a) The structure and synthetic method for rCTF, (b) the electrochemical performance of rCTF and (c) the simulated lithium storage mechanism[69] (Reproduced by permission of Wiley-VCH).

    Figure  4.  (a) The synthetic route of TFPB-COF, (b) the electrochemical performance of TFPB-COF and (c) the lithium storage mechanism[88] (Reproduced by permission of Wiley-VCH).

    Figure  5.  The relationship between voltage and molecular structure: (a) small molecules as the cathode in a LIB: molecular structures, differential capacity curves and correlation between the first reduction potentials and the calculated LUMO energies[94], (b) the effect of active sites position[95] and (c) conjugated structure[96] on voltage ((a) Reproduced by permission of Wiley-VCH, (b) Reproduced by permission of American Chemical Society and (c) Reproduced by permission of the Royal Society of Chemistry.

    Figure  6.  (a) Different molecular configurations, (b) the electrochemical performance of three COFs, (c) the molecular orbital energy level of three different COFs[79] (Reproduced by permission of the Royal Society of Chemistry).

    Figure  7.  (a) The microstructures of two COFs, (b) the specific capacity, the cyclic voltammetry curves for (c) Tp-DANT-COF and (d)Tb-DANT-COF[64] (Reproduced by permission of the Royal Society of Chemistry).

    Figure  8.  (a) The structure of a nitrogen-rich COF, (b) the rate performance, (c) the cyclic voltammetry curves for the nitrogen-rich COF and (d) lgi-lgv curves for the b evaluation[53] (Reproduced by permission of Nature Publishing Group).

    Figure  9.  (a) The synthetic route of TpBpy-COF, (b) the XRD pattern of TpBpy-COF and (c) cyclic performance of TpBpy-COF[84] (Reproduced by permission of Wiley-VCH).

    Figure  10.  (a) Structures of DAAQ-COF with different thicknesses, (b) change of EPR signal for COFs with different thicknesses and (c) the cyclic performance for DAAQ-COF with a thickness of 4-12 nm[67] (Reproduced by permission of American Chemical Society).

    Figure  11.  (a) Synthesis of AQ-COF@CNTs, (b) the cyclic performance of AQ-COF@CNTs and (c) lgi-lgv curves[75] (Reproduced by permission of the Royal Society of Chemistry).

    Table  1.   The representative COF electrode materials in RMBs.

    COFs’ nameApplication
    Scenarios
    Current density (mA g−1)/
    Specific capacity (mAh g−1)
    Voltage
    Window (V)
    Lifespan (cycles)/
    Capacity retention (%)
    Current density (A g−1)/
    Specific capacity (mAh g−1)
    Ref.
    DTP–ANDI–COF@CNTLIB200/701.5−3.5700/1001/60[52]
    PIBN-COF@GrapheneLIB28/2711.5−3.5300/862.8/200[54]
    DAAQ-TFP–COFLIB20/1101.5−41000/1003/20[66]
    DAAQ-ECOFLIB20/1451.5−41800/1003/50[66]
    DAAQ-COFSIB100/4200.05−310000/995/200[67]
    DABQ-ECOFLIB20/~2001.5−3.5//[66]
    TEMPO–ECOFLIB20/~1002−4//[66]
    TQBQ-COFSIB20/3501−3.61000/9610/134[53]
    TRO–COFLIB27.4/2680.5−4.5100/99.90.548/100[62]
    N2–COFLIB1000/7000.05−3500/755/500[68]
    N3–COFLIB1000/7000.05−3500/655/550[68]
    Tp-DANT-COFLIB200/78.91.5−4600/902/70[64]
    Tb-DANT-COFLIB50/1351.5−4300/832/67[64]
    rCTFLIB300/11900.005−31500/10012/500[69]
    PI-ECOF-1LIB14.2/1121.5−3.5300/750.284/70[65]
    PI-ECOF-2LIB12.8/1031.5−3.5300/750.256/40[65]
    TFPB-TAPT COFSIB30/2000.05−1.6500/50.80.2/145[70]
    BQ1-COFLIB39/5021.2−3.51000/817.73/171[71]
    C2N-450LIB37.2/9330.02−3500/130.63.72/40.1[72]
    C3NLIB37.2/7870.02−3500/913.72/180[72]
    PGF-1LIB500/4801−3.51400/78.35/200[73]
    DBA-COF 3LIB50/2000.05−390/1001/90[74]
    AQ-COF@CNTLIB50/711.5−3.53000/1002.5/11[75]
    TThPPLIB1000/4000.005−3200/1004/200[60]
    JUC-526LIB200/441.20.01−3500/1002/200[76]
    HATN-CMPLIB100/1501.5−450/601/50[77]
    IISERP-CON1LIB100/7200.01−31000/1002/460[78]
    IISERP-COF16SIB100/800.01−3500/100/[79]
    IISERP-COF17SIB100/2000.01−3500/1001/100[79]
    IISERP-COF18SIB100/4000.01−31400/9215/127[79]
    Pa-COFLIB1000/401.30.01−3.52000/74.85/141.8[80]
    Tb-COFLIB1000/379.10.01−3.52000/72.75/144[80]
    TAPB-terephthal Aldehyde COFsSIB100/3030−31000/855/150[81]
    Cz-COF1LIB200/3000.01−3400/591/200[82]
    Cz-COF2200/250400/501/100[82]
    Tp-Azo-COFLIB1000/3060.01−33000/1002.4/100[83]
    TpBpyAIB2000/1500.01−2.313000/1005/113[84]
    CTF-0KIB100/1000.01−3350/671/63[85]
    CTF-1100/50350/671/31[85]
    DAPT-TFP-CPFSIB100/1500.8−3.21400/94.75/100[86]
    PDI-TcLIB190/451.8−3.2500/800.482/22[87]
    HqTp-COFZIB625/1500.2−1.81000/951.25/125[56]
    COF-CNTLIB100/15360.005−3500/5105/200[54]
    2D CCP-HATNLIB500/1161.2−3.91000/911/94[55]
    E-CIN-1/CNTLIB100/5380.001−3250/1245/97[58]
    E-SNW-1/CNT100/542250/915/212[58]
    COF-10@CNTKIB100/2880.005−34000/545/68[59]
    E-TFPB-COF/MnO2LIB100/12500.005−3300/1355/500[88]
    Si@COFLIB1000/20000.01−11000/605/1000[89]
    下载: 导出CSV
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  • 收稿日期:  2021-01-11
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