Volume 38 Issue 5
Oct.  2023
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Article Navigation >  New Carbon Mater.  > 2023  >  38(5): 787-803
WANG Ji-rui, YANG Da-hai, XU Yi-jian, HOU Xiang-long, EDISON Huixiang Ang, WANG De-zhao, ZHANG Le, ZHU Zhen-dong, FENG Xu-yong, SONG Xiao-hui, XIANG Hong-fa. Recent developments and the future of the recycling of spent graphite for energy storage applications. New Carbon Mater., 2023, 38(5): 787-803. doi: 10.1016/S1872-5805(23)60777-2
Citation: WANG Ji-rui, YANG Da-hai, XU Yi-jian, HOU Xiang-long, EDISON Huixiang Ang, WANG De-zhao, ZHANG Le, ZHU Zhen-dong, FENG Xu-yong, SONG Xiao-hui, XIANG Hong-fa. Recent developments and the future of the recycling of spent graphite for energy storage applications. New Carbon Mater., 2023, 38(5): 787-803. doi: 10.1016/S1872-5805(23)60777-2
shu

Recent developments and the future of the recycling of spent graphite for energy storage applications

doi: 10.1016/S1872-5805(23)60777-2
  • 1.

    School of Materials Science and Engineering, Hefei University of Technology, Hefei 230009, China

  • 2.

    Natural Sciences and Science Education, National Institute of Education, Nanyang Technological University 637616, Singapore

  • 3.

    Hefei Gotion High-Tech Power Energy Co., Ltd, Hefei, Anhui 230012, China

  • 4.

    Intelligent Manufacturing Institute, Hefei University of Technology, Hefei 230051, China

Funds:  This work was supported by the National Natural Science Foundation of China (52072105), the Anhui Provincial Natural Science Foundation (2108085J23 and 2208085QE134), Key R&D Program of Anhui Province (2021e03020001 and 202104a05020044), the Start-up grant from Hefei University of Technology (13020-03712021026), and the Academic Research Fund (RI 1/21 EAH) of the National Institute of Education, Singapore
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  • Author Bio:

    王继锐，硕士研究生. E-mail：19810931417@163.com

  • Corresponding author: SONG xiao-hui, Associate professor. E-mail: xiaohuisong@hfut.edu.cn; XIANG hong-fa, Professor. E-mail: hfxiang@hfut.edu.cn
  • Received Date: 2023-05-31
  • Accepted Date: 2023-07-07
  • Rev Recd Date: 2023-07-06
    • Available Online: 2023-08-28
  • Publish Date: 2023-10-01
    Abstract
  • This review provides an extensive analysis of the recycling and regeneration of battery-grade graphite obtained from used lithium-ion batteries. The main objectives are to address supply-demand challenges and minimize environmental pollution. The study focuses on the methods involved in obtaining, separating, purifying, and regenerating spent graphite to ensure its suitability for high-quality energy storage. To improve the graphite recovery efficiency and solve the problem of residual contaminants, techniques like heat treatment, solvent dissolution, and ultrasound treatment are explored. Wet and pyrometallurgical purification and regeneration methods are evaluated, considering their environmental impact and energy consumption. Sustainable and cost-effective approaches, including acid-free purification and low-temperature graphitization, are highlighted. Specific requirements for regenerated graphite in lithium-ion batteries and supercapacitors are discussed, emphasizing customized recycling processes involving acid leaching, high-temperature treatment, and surface coating. Valuable information for the development of efficient and sustainable energy storage systems is provided, addressing environmental issues, and how to meet the increasing demand for graphite anodes.
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