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纳米碳基表面分子印迹吸附剂综述及其吸附机理探讨

秦蕾 刘伟峰 刘旭光 杨永珍 张立安

秦蕾, 刘伟峰, 刘旭光, 杨永珍, 张立安. 纳米碳基表面分子印迹吸附剂综述及其吸附机理探讨[J]. 新型炭材料, 2020, 35(5): 459-485. doi: 10.1016/S1872-5805(20)60503-0
引用本文: 秦蕾, 刘伟峰, 刘旭光, 杨永珍, 张立安. 纳米碳基表面分子印迹吸附剂综述及其吸附机理探讨[J]. 新型炭材料, 2020, 35(5): 459-485. doi: 10.1016/S1872-5805(20)60503-0
QIN Lei, LIU Wei-feng, LIU Xu-guang, YANG Yong-zhen, ZHANG Li-an. A review of nanocarbon-based molecularly imprinted polymer adsorbents and their adsorption mechanisms[J]. NEW CARBOM MATERIALS, 2020, 35(5): 459-485. doi: 10.1016/S1872-5805(20)60503-0
Citation: QIN Lei, LIU Wei-feng, LIU Xu-guang, YANG Yong-zhen, ZHANG Li-an. A review of nanocarbon-based molecularly imprinted polymer adsorbents and their adsorption mechanisms[J]. NEW CARBOM MATERIALS, 2020, 35(5): 459-485. doi: 10.1016/S1872-5805(20)60503-0

纳米碳基表面分子印迹吸附剂综述及其吸附机理探讨

doi: 10.1016/S1872-5805(20)60503-0
基金项目: 国家自然科学基金(21706170,U1610255,U1607120,51902222);澳大利亚研究委员会产业转化研究项目(IH170100009);山西省重点研发国际合作项目(201903D421077);科技部国家重点研发计划(2017YFB0603104);山西省自然科学基金(201801D221077);山西省科技创新重点团队(201605D131045-10);山西省高校科技创新项目(2020L0097,2019L0255).
详细信息
    通讯作者:

    刘旭光,教授.E-mail:liuxuguang@tyut.edu.cn

  • 中图分类号: TQ127.1+1

A review of nanocarbon-based molecularly imprinted polymer adsorbents and their adsorption mechanisms

Funds: The authors are grateful for the financial support from the National Natural Science Foundation of China (Nos. 21706170, U1610255, U1607120, 51902222), the Australian Research Council (ARC) Industrial Transformation Research Hub (IH170100009), Key R&D Program of Shanxi Province (International Cooperation, 201903D421077), the National Key Research and Development Program of China (2017YFB0603104), Shanxi Province Natural Science Foundation (201801D221077), the Shanxi Provincial Key Innovative Research Team in Science and Technology (201605D131045-10), the Scientific and Technological Innovation Programs of Higher Education Institutions in Shanxi (2020L0097, 2019L0255). And the first author would like to appreciate the allowance support from China Scholarship Council.
  • 摘要: 纳米碳基材料由于具有低密度、高强度、环境友好、结构可控、表面易于修饰等优点,成为了一类非常理想的表面分子印迹基质材料。相应的纳米碳基表面分子印迹聚合物(C-SMIPs)吸附剂,对于实现液相环境体系中的有机小分子污染物的选择性吸附脱除与富集回收取得了令人满意的效果。本综述对该应用背景下近五年来的不同维度C-SMIPs进行了归纳总结。不仅发现C-SMIPs吸附能力的下限更容易受基质材料的影响,其上限则更多地取决于印迹层的构建情况,以多孔纳米炭球和氧化石墨烯为基质的C-SMIPs通常具有较高的吸附容量,其中氧化石墨烯基SMIPs通常具有较高的吸附效率。同时本综述还推断出C-SMIPs对于目标分子吸附的本质是固液界面间的物理性吸附,解决了长时间以来令人困扰的对吸附过程定性的争议。另外,通过本综述的探讨分析,可以为接下来深入研究C-SMIPs的基质筛选、印迹方法、吸附条件选择等提供一些可借鉴的理论和实践经验,从而不断推进C-SMIPs的研发和应用。
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  • 收稿日期:  2020-08-26
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