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Recent progress in MXene-based nanomaterials for high-performance aqueous zinc-ion hybrid capacitors

ZHANG Ming-hui XU Wen WU Li-sha DONG Yan-feng

张明慧, 徐文, 武丽莎, 董琰峰. MXene基纳米材料在高性能水系锌离子混合电容器中的研究进展. 新型炭材料(中英文), 2022, 37(3): 508-526. doi: 10.1016/S1872-5805(22)60611-5
引用本文: 张明慧, 徐文, 武丽莎, 董琰峰. MXene基纳米材料在高性能水系锌离子混合电容器中的研究进展. 新型炭材料(中英文), 2022, 37(3): 508-526. doi: 10.1016/S1872-5805(22)60611-5
ZHANG Ming-hui, XU Wen, WU Li-sha, DONG Yan-feng. Recent progress in MXene-based nanomaterials for high-performance aqueous zinc-ion hybrid capacitors. New Carbon Mater., 2022, 37(3): 508-526. doi: 10.1016/S1872-5805(22)60611-5
Citation: ZHANG Ming-hui, XU Wen, WU Li-sha, DONG Yan-feng. Recent progress in MXene-based nanomaterials for high-performance aqueous zinc-ion hybrid capacitors. New Carbon Mater., 2022, 37(3): 508-526. doi: 10.1016/S1872-5805(22)60611-5

MXene基纳米材料在高性能水系锌离子混合电容器中的研究进展

doi: 10.1016/S1872-5805(22)60611-5
基金项目: 辽宁省“兴辽英才计划”青年拔尖人才(XLYC2007129); 辽宁省自然科学基金(2020-MS-095);中央高校基本科研业务费(N2105008);中国科学院炭材料重点实验室开放课题(KLCMKFJJ2004)
详细信息
    通讯作者:

    董琰峰,副教授. E-mail:dongyanfeng@mail.neu.edu.cn

  • 中图分类号: TB33

Recent progress in MXene-based nanomaterials for high-performance aqueous zinc-ion hybrid capacitors

Funds: This work was financially supported by LiaoNing Revitalization Talents Program (XLYC2007129), the Natural Science Foundation of Liaoning Province (2020-MS-095), the Fundamental Research Funds for the Central Universities of China (N2105008), and the CAS Key Laboratory of Carbon Materials (KLCMKFJJ2004)
More Information
    Author Bio:

    张明慧、徐文为共同第一作者

    Corresponding author: DONG Yan-feng, Associate Professor. E-mail: dongyanfeng@mail.neu.edu.cn
  • 摘要: 水系锌离子混合电容器(ZHCs)具有本征安全、低成本的优点,在大规模储能领域中具有广阔的应用前景。然而,传统的多孔炭正极具有不理想的孔结构,难以实现有效的锌离子的存储和扩散,此外锌箔负易遭受枝晶和副反应,因此传统ZHCs常表现出较低的能量密度和较短的循环寿命,严重制约其实际应用。二维过渡金属碳/氮化物(MXene)具有高导电基体和丰富表面官能团,为构筑ZHCs用高容量正极和长循环锌负极提供了新机遇。本文系统总结了高性能ZHCs用MXene基纳米材料的最新进展,先简要介绍了ZHCs的基础知识如工作原理和关键电化学参数,随后详细阐述了高性能ZHCs用MXene基正极(纯MXene、插层MXene、掺杂MXene、MXene基杂化材料(MXene/金属硫化物、MXene/炭、MXene/聚合物))和负极的研究进展,最后简要讨论了MXene基纳米材料在下一代ZHCs应用中的挑战和展望。
  • FIG. 1535.  FIG. 1535.

    FIG. 1535.. 

    Figure  1.  Main progress of MXene-based nanomaterials for ZHCs. (a) MXene was firstly obtained by selective etching of Al in Ti3AlC2 with HF acid[42] (Reprinted with permission by copyright 2011, Wiley). (b) MXene-reduced graphene oxide aerogels as the cathode[32](Reprinted with permission by copyright 2019, Wiley). (c) Sn4+ pre-embedded MXene cathode[33] (Reprinted with permission by copyright 2020, Wiley). (d) Nitrogen-doped MXene-based heterostructure cathode[34] (Reprinted with permission by copyright 2021, RSC). (e) Nanofibrillated cellulose adhered Ti3C2Tx flake cathode[35](Reprinted with permission by copyright 2022, Elsevier). (f) Zn nanosheets vertically deposited on Ti3C2 MXene [36] (Reprinted with permission by copyright 2019, ACS). (g) Ti3C2Tx MXene paper host for Zn [37] (Reprinted with permission by copyright 2021, ACS). (h) Heterolayer of MXene and ZnS on Zn[38] (Reprinted with permission by copyright 2021, ACS). (i) Ti3C2Tx MXene wrapped Zn powder[39] (Reprinted with permission by copyright 2021, ACS).

    Figure  2.  Schematic diagram of the applications of MXene based nanomaterials for aqueous zinc-ion hybrid capacitors.

    Figure  3.  Schematic of the storage mechanisms of (a) electric double layer capacitance, (b) redox pseudocapacitance, and (c) intercalation pseudocapacitance[44](Reprinted with permission by copyright 2021, Wiley). (d-e) Schematic diagrams of energy storage mechanisms of (d) the first type and (e) the second type ZHCs.

    Figure  4.  (a) Schematic diagram of 3DP MXene electrodes. (b) SEM image of 3DP MXene. (c) Specific capacitances based on mass and area at different current densities[62](Reprinted with permission by copyright 2021, ACS). (d) Schematic diagram of the preparation process of diamine-intercalated MXene. (e) SEM image of PDA-MXene. (f) Specific capacitances of MXene electrodes intercalated with different diamine molecules at different current densities. (g) Cycling performance of PDA-MXene electrodes at 1 A g−1[64](Reprinted with permission by copyright 2021, Wiley).

    Figure  5.  (a) Schematic diagram of preparation of Ti3C2Tx/BiCuS2.5. (b) Ragone plot of Ti3C2Tx/BiCuS2.5 and other reported electrodes. (c) Cycling performance of Ti3C2Tx/BiCuS2.5 electrodes at a current density of 20 A g−1[67](Reprinted with permission by copyright 2021, Elsevier).

    Figure  6.  (a) Schematic of the synthesis of V2C@CNTs. (b) SEM image of V2C@CNTs[68](Reprinted with permission by copyright 2019, Wiley). (c) SEM image of MXene-rGO[32] (Reprinted with permission by copyright 2019, Wiley). (d) Schematic of the synthesis of NMXC[34] (Reprinted with permission by copyright 2021, RSC).

    Figure  7.  (a) Schematic diagram of the preparation of a flexible layered Ti3C2Tx MXene@Zn paper. (b) Coulombic efficiency of Zn plating/stripping of Zn|Ti@Zn batteries and Zn|MXene@Zn batteries at an areal capacity of 1 mAh cm−2 and a current density of 1 mA cm−2[37](Reprinted with permission by copyright 2021, ACS). (c) Cycling performance of Zn//Ti3C2I2 and MCl-Zn//Ti3C2I2 batteries at a current density of 3 A g−1[82]. (Reprinted with permission by copyright 2022, ACS).

    Figure  8.  (a) Schematic of the synthesis of S/MX@ZnS@Zn. (b) Cycling performance of pristine Zn and S/MX@ZnS@Zn anodes at a rate of 0.5 mA cm−2 and an areal capacity of 0.5 mAh cm−2. SEM images of (c) pristine Zn anodes and S/MX@ZnS@Zn-350 anodes after 10 and 100 cycles[38] (Reprinted with permission by copyright 2021, ACS). (d) SEM image of MXene@Zn. (e) Nucleation overpotential of Zn-p and MXene@Zn at 1mA cm−2. (f) Long-cycle performance diagram of Zn-p and MXene@Zn symmetric batteries at 1 mA cm−2[39](Reprinted with permission by copyright 2021, ACS).

    Table  1.   A summary of various reported MXene based cathodes for ZHCs.

    Type of cathodeSampleVoltage (V)ElectrolyteCapacityCapacity retentionEnergy densityPower densityRef.
    MXenesTi3C2Tx0.05-1.352 M ZnSO4132 F g−1 at 0.5 A g−182.5% after 1000 cycles[36]
    Mo1.33CTz-Ti3C2Tz0.01-1.33 M Zn(CF3SO3)2115 mAh g−1 at 1 A g−190% after 8000 cycles103 Wh kg−10.143 KW kg−1[60]
    3D-PHMF0-1.32 M Zn(CF3SO3)2105.6 mAh g−1 at 0.2 A g−190% after 20000 cycles53.6 Wh kg−1104.5W kg−1[61]
    3DP MXene0.1-1.22 M ZnSO4259.7 F g−1 at 0.1 A g−186.5% over 6000 cycles0.10 mWh cm−25.90 mW cm−2[62]
    Ti3C2Tx (Fiber-
    shaped ZHCs )
    0-1.21.5 M ZnSO4214 mF cm−2 at 5 mV s−183.58% after 5000 cycles42.8 μWh cm−20.64 mW cm−2[63]
    Intercalated
    MXenes
    PDA-MXene0.2-1.12 M ZnSO4124.4 F g−1 at 0.2 A g−185% after 10000 cycles13.8 Wh kg−14500 W kg−1[64]
    In-situ pillared Ti3C20.2-1.20.1 M ZnSO473 mAh g−1 at 0.2 A g−196% after 1000 cycles[65]
    Sn4+-Ti2CTx/C0.1-2.02 M ZnSO4138 mAh g−1 at 0.1 A g−1>96% after 12500 cycles[33]
    Heteroatom-doped
    MXenes
    N-Ti3C20.05-1.21 M ZnSO4247.9 F g−1 at 0.1 A g−188.34% after 6000 cycles45.54 Wh kg−14093 W kg−1[66]
    MXene/metal
    sulfide hybrids
    Ti3C2Tx/
    Bi2S3@N-C
    0-1.4ZnSO4653 F g−1 at 1 A g−185.7% after 2000 cycles46.98 Wh kg−1750 W kg−1[51]
    Ti3C2Tx/BiCuS2.50-0.81 M ZnSO4840 C g−1 at 1 A g−182% after 10000 cycles298.4 Wh kg−17200 W kg−1[67]
    MXene/carbon
    hybrids
    V2C/CNTs0.1-1.11 M ZnSO490.2 F g−1 at 10 A g−1[68]
    MXene-rGO0.2-1.62 M ZnSO4128.6 F g−1 at 0.4 A g−195% after 75000 cycles34.9 Wh kg−1279.9 W kg−1[32]
    NMXC0.2-1.82 M ZnSO483.9 mAh g−1 at 0.1 A g−196.4 % after 10000 cycles64.5 Wh kg−13.9 kW kg−1[34]
    MXene/polymer
    hybrids
    MN-802 M ZnSO492.1 mAh g−1
    at 0.5 mA cm−2
    94.31% after 10000 cycles[35]
    MXene/BCF0-1.22 M Zn(CF3SO3)2
    /PAM gel
    178.6 mF cm−2

    at 0.5 mA cm−2
    72.3% after 3000 cycles34.0 μWh cm−2[69]
    MXene/BC@PPy0-1.92 M Zn(CF3SO3)2-0.1 M MnSO4/PAM
    hydrogel
    388 mF cm−2 at 1 mA cm−295.8% after 25000 cycles145.4 μWh cm−23.78 mW cm−2[70]
    Note: M: mol L−1
    下载: 导出CSV

    Table  2.   A summary of various reported MXene-based anodes for ZHCs.

    Role of MXenesAnode nameVoltage hysteresisNucleation overpotentialLife spanCoulombic efficiencyRef.
    Zn host materialsTi3C2Tx MXene@Zn75 mV
    (1 mA cm−2)
    83 mV300 h
    (1 mA cm−2)
    94.13% at 5 mA cm−2 (400 cycles)[37]
    MCl-Zn103 mV
    (10 mA cm−2)
    40.7 mV
    (1 mA cm−2)
    840 h
    (2 mA cm−2)
    99.50% at 1 mA cm−2 (50 cycles)[82]
    MGA@Zn64 mV
    (10 mA cm−2)
    1050 h
    (10 mA cm−2)
    ≈99.67% at 10 mA cm−2 (600 cycles)[83]
    Protecting layersS/MX@ZnS@Zn-3500.03 V
    (0.5 mA cm−2)
    1600 h
    (10 mA cm−2)
    [38]
    MXene-mPPy/Zn22 mV
    (0.2 mA cm−2)
    10 mV2500 h
    (0.2 mA cm−2)
    [84]
    AMX-Zn[81]
    MXene@Zn (Zn-p)30 mV
    (1 mA cm−2)
    27.4 mV
    (1 mA cm−2)
    200 h
    (1 mA cm−2)
    [31]
    下载: 导出CSV
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  • 收稿日期:  2022-03-02
  • 修回日期:  2022-04-19
  • 网络出版日期:  2022-04-27
  • 刊出日期:  2022-06-01

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